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lpetrich
01 Apr 2009, 07:29 PM
The RNA world hypothesis states that the DNA-RNA-protein organisms of the present-day world had some ancestors in which RNA both transmitted genetic information and acted as enzymes.

This hypothesis is partially motivated by the chicken-and-egg conundrum presented by the DNA-RNA-protein system. DNA contains master copies of genetic information, RNA contains intermediate copies and assists in assembling proteins, and proteins due most of the catalytic and structural work. In fact, proteins do nearly all the work of assembling the building blocks of all the macromolecules.

But can this system be simplified? It looks like an excellent example of irreducible complexity, a multipart system whose parts cannot function in isolation. However, it has often been possible to find intermediates that can easily be modified to yield the irreducibly-complex system. A parallel macroscopic system is honeybee societies, where queens are dependent on workers for just about everything, including founding new hives. But in many species, like bumblebees, lone queens found hives and raise the first generation of workers. So if queens start taking workers with them to found hives, one gets the honeybee swarming approach.

Proteins?

They are very versatile molecules, but it is hard to create a self-replicating protein. It is much easier with nucleic acids; in fact, Watson and Crick first recognized a simple mechanism for that when they worked out the double-helix structure of DNA in 1951-1953.

DNA?

It is more chemically stable than RNA, but it is only used as a master copy. So a DNA-first approach would have required replacement of DNA in all but one function, without leaving any vestigial uses behind.

RNA?

Unlike DNA, and despite its lesser chemical stability, it has several functions.

Messenger RNA

It carries a gene sequence from the genome to the ribosomes, which act as workbenches for assembling proteins.

Transfer RNA

One end is for matching the messenger RNA, and the other end is for holding the amino acid for a protein.

Ribosomal RNA

These molecules are the most essential part of ribosomes, with ribosomal proteins mainly acting as scaffolding.

Stray RNA

There are lots of bits of RNA that appear in contexts where one may not expect RNA to be present. These are reasonably interpreted as vestigial features of a former RNA world.

A short strand of RNA is needed as a primer for the enzyme DNA polymerase, which helps assemble DNA molecules (why RNA and not DNA?).

Bits of RNA are present in several cofactors, molecules that work with enzymes, like

NAD, NADP (electron transfer; can add/subtract hydrogen)
FAD, FMN (electron transfer; can add/subtract hydrogen)
Coenzyme A (acetate)
Vitamin B12 (methyl groups)

An RNA nucleotide is present in the energy intermediate ATP (adenosine triphosphate); the energy is in the phosphate-phosphate bonds and the adenosine is most likely a handle for the enzymes that work with it.

DNA nucleotides are all made from RNA ones, by turning an -OH into a -H in the ribose, and then adding a methyl group to the uracil to make thymine.

Ribozymes

In the 1980's, Thomas Cech was researching RNA splicing, and in 1986, he discovered some RNA that could splice itself without any assistance from any proteins. This startling discovery won him a Nobel Prize in 1989. Since then, several other ribozymes have been both discovered and made in labs. Ribosomes have also turned out to be a kind of ribozyme.

No DNA counterparts, deoxyribozymes or DNAzymes, have ever been found in the wild; they have all been made in various labs.

RNA-world Metabolism and Biosynthesis

One can identify some RNA-world metabolic capabilities, notably electron transfer (reduction-oxidation or redox reactions), methyl-group transfer, acetyl-group transfer, etc.

Many RNA-world ribozymes likely had some modified bases, which likely broadened their catalytic capabilities. One can reasonably infer this from the modified RNA bases of our world, notably in transfer RNA. In that molecule, uridine (uracil+ribose) gets turned into pseudouridine in a few spots, some of its adenines sometimes get turned into inosine, etc. Likewise, the niacin part of NAD looks like a modified nucleic-acid base.

Departing from the RNA World

There were two main steps needed to depart from it: the development of DNA and the development of proteins.

DNA is a modification of RNA, one that is only used for master copies of genetic information. In fact, the authors of Did DNA replication evolve twice independently? (http://www.ncbi.nlm.nih.gov/pubmed/10446225) propose that the evolution of DNA replication had been incomplete when the ancestors of Bacteria and Archaea/Eukarya split. They propose that their most recent ancestor had a DNA-RNA genome, with replication by both DNA -> RNA and RNA -> DNA copying. Early Bacteria and Archaea/Eukarya then separately elaborated on this system to produce the DNA -> DNA systems of today.

Amino acids, the building blocks of proteins, likely started out as cofactors of ribozymes. But along the way, the ribozymes built fancier and fancier multi-amino-acid cofactors until those cofactors took over and became the primary enzymes. Thus, proteins emerged. And some of the protein-assembly ribozymes have survived as ribosomes.

Before the RNA World?

The RNA-world hypothesis does not address the question of its origin; we must turn to prebiotic chemistry for answers to that. In experiments with such chemistry, RNA bases can be readily formed, but ribose requires relatively unusual conditions.

For that reason, there has been work on possible RNA ancestors like pyranosyl RNA (p-RNA) and Peptide Nucleic Acids (PNA), which use something other than ribose as their "backbone" molecule. So the first organism could have been a p-RNA or a PNA one or some other such, with RNA resulting from ribose getting substituted for the original "backbone" molecule.

Although the origin of life continues to be an unsolved problem, the "RNA world" hypothesis significantly narrows the gap between known prebiotic chemistry and the first organisms.

premjan
01 Apr 2009, 08:13 PM
I like the dual origin hypothesis better than the RNA world, though I think RNA did precede DNA.

Codec
02 Apr 2009, 07:49 AM
There are problems with an RNA world. RNA is rather unstable on its own, the OH group at position 2 will tend to attack the 3C in a nucleophilic reaction, if it gets the chance, leading to the molecule cutting itself into pieces. Apparently having it folded helps stabilise again this sort of attack.
DNA doesn't have that group (hence the deoxy) so is far more stable.

Steviepinhead
02 Apr 2009, 11:24 PM
I like the dual origin hypothesis better than the RNA world, though I think RNA did precede DNA.
I had to work harder than usual to find the buried pun in there:
precede ==> pre-seed

:bang:

premjan
03 Apr 2009, 12:55 AM
I didn't mean it as a pun.

epepke
03 Apr 2009, 04:40 AM
You didn't mention the big problem with a DNA origin, which is the topology of DNA.

Hmm... there doesn't seem to be a Wikipedia entry for topases.

Steviepinhead
03 Apr 2009, 09:48 PM
I didn't mean it as a pun.

I know. :notworthy: But that would neatly explain why I had to work so hard to unearth it! :cool:

lpetrich
03 Apr 2009, 10:47 PM
You didn't mention the big problem with a DNA origin, which is the topology of DNA.

Hmm... there doesn't seem to be a Wikipedia entry for topases.
Are you talking about topoisomerase enzymes?

These enzymes make one strand of DNA cross another by snipping it to allow the other strand to pass, then rejoining it.

epepke
04 Apr 2009, 01:06 AM
You didn't mention the big problem with a DNA origin, which is the topology of DNA.

Hmm... there doesn't seem to be a Wikipedia entry for topases.
Are you talking about topoisomerase enzymes?

These enzymes make one strand of DNA cross another by snipping it to allow the other strand to pass, then rejoining it.

Yes. DNA would be a non-starter without them.

lpetrich
07 Apr 2009, 07:16 AM
I decided to take another look at the paper Modern metabolism as a palimpsest of the RNA world (http://www.pnas.org/content/86/18/7054.abstract). It came out in 1989, 20 years ago, so it's likely a bit out of date by now. In particular, it treats Archaea, Bacteria, and Eukarya as coequals, when Eukarya is largely a hybrid of various prokaryotes. So here's what likely evolved when:

Tetrapyrroles. They appear in chlorophyll, heme, vitamin B12, methanogen coenzyme F430, etc. They have two different biosynthesis pathways leading to 5-aminolevulinate, the Shemin (glycine + succinyl CoA) and the C5 (glutamate).

The C5 pathway is found in archaea, most bacteria, and plants, while the Shemin one is found in alpha-proteobacteria and non-plant eukaryotes. Interestingly, Euglena gracilis has both, C5 in its chloroplasts and Shemin in the rest of the cell (evidence of Shemin (http://www.pubmedcentral.nih.gov/articlerender.fcgi?artid=319193) and evidence of C5 (http://www.pubmedcentral.nih.gov/articlerender.fcgi?artid=1081127)). The Euglena chloroplast is a (eukaryotic) green alga that one of its ancestors "ate" and turned into a chloroplast.

The authors of Evolutionary relationship between initial enzymes of tetrapyrrole biosynthesis (http://www.ncbi.nlm.nih.gov/pubmed/16564539) propose that one of the Shemin-pathway enzymes had evolved from one of the C5-pathway enzymes, suggesting that the Shemin one was invented in some early alpha-proteobacterium. Mitochondria are descended from alpha-proteobacteria, and their endosymbiosis thus transmitted the Shemin pathway to eukaryotes. However, chloroplasts carried the C5 pathway with them, making plants use C5 instead of Shemin.

So one concludes that the C5 pathway is the ancestral one. It has a curious feature: the glutamate is contributed while attached to a transfer RNA. This suggests that this pathway goes all the way back to the RNA world.

This RNA-world ancestry is also consistent with the putative RNA-world ancestry of vitamin B12.

Turning to coenzyme F430, it is involved in methanogens' methane production, along with coenzyme M and methanfuran. None of these contain RNA, however, suggesting that methanogens' methane production is likely a later invention.

Fatty Acids. These are present only in Bacteria and Eukarya, and in the latter, their biosynthesis may have been an import from the former. The palimpsest-paper authors argue that fatty acids are a post-protein latecomer. Their biosynthesis enzymes have a lot of variation, and their biosynthesis involves Acyl Carrier Protein (a protein, of course), and biotin (apparently post-protein).

Terpenes. These are polymers of isoprene, and they are made in very similar fashion across all three domains, though they are more difficult to trace back to the RNA world than tetrapyrroles. They are found in numerous places, like in the cell membranes of Archaea, and they may have been the original cell-membrane lipids.


Summary of where/when each one likely originated:

Tetrapyrroles: RNA world
Fatty acids: ancestor of Bacteria
Terpenes: before Bacteria - Archaea split


Turning to enzyme cofactors again, for a more detailed discussion of them, see Cofactor (biochemistry). And as to cofactor vs. coenzyme,

Loosely-bound: coenzymes
Tightly-bound: prosthetic groups